Unleashed was released on May 12, 2010 and has a total of 96 cards (95 regular/1 secret) in the set.
| Num | Name | Type | HP | Rarity | |
|---|---|---|---|---|---|
| TWO | Alph Lithograph | Trainer - Item | Rare Secret | ||
| 1 | Jirachi | Pokémon - Basic | 60 | Rare Holo | |
| 2 | Magmortar | Pokémon - Stage 1 | 110 | Rare Holo | |
| 3 | Manaphy | Pokémon - Basic | 60 | Rare Holo | |
| 4 | Metagross | Pokémon - Stage 2 | 130 | Rare Holo | |
| 5 | Mismagius | Pokémon - Stage 1 | 90 | Rare Holo | |
| 6 | Octillery | Pokémon - Stage 1 | 80 | Rare Holo | |
| 7 | Politoed | Pokémon - Stage 2 | 120 | Rare Holo | |
| 8 | Shaymin | Pokémon - Basic | 70 | Rare Holo | |
| 9 | Sudowoodo | Pokémon - Basic | 90 | Rare Holo | |
| 10 | Torterra | Pokémon - Stage 2 | 140 | Rare Holo | |
| 11 | Xatu | Pokémon - Stage 1 | 90 | Rare Holo | |
| 12 | Beedrill | Pokémon - Stage 2 | 110 | Rare | |
| 13 | Blastoise | Pokémon - Stage 2 | 130 | Rare | |
| 14 | Crobat | Pokémon - Stage 2 | 110 | Rare | |
| 15 | Fearow | Pokémon - Stage 1 | 80 | Rare | |
| 16 | Floatzel | Pokémon - Stage 1 | 80 | Rare | |
| 17 | Kingdra | Pokémon - Stage 2 | 130 | Rare | |
| 18 | Lanturn | Pokémon - Stage 1 | 90 | Rare | |
| 19 | Lucario | Pokémon - Stage 1 | 90 | Rare | |
| 20 | Ninetales | Pokémon - Stage 1 | 90 | Rare | |
| 21 | Poliwrath | Pokémon - Stage 2 | 130 | Rare | |
| 22 | Primeape | Pokémon - Stage 1 | 90 | Rare | |
| 23 | Roserade | Pokémon - Stage 1 | 90 | Rare | |
| 24 | Steelix | Pokémon - Stage 1 | 120 | Rare | |
| 25 | Torkoal | Pokémon - Basic | 80 | Rare | |
| 26 | Tyranitar | Pokémon - Stage 2 | 140 | Rare | |
| 27 | Ursaring | Pokémon - Stage 1 | 100 | Rare | |
| 28 | Cherrim | Pokémon - Stage 1 | 80 | Uncommon | |
| 29 | Dunsparce | Pokémon - Basic | 60 | Uncommon | |
| 30 | Golbat | Pokémon - Stage 1 | 80 | Uncommon | |
| 31 | Grotle | Pokémon - Stage 1 | 90 | Uncommon | |
| 32 | Kakuna | Pokémon - Stage 1 | 80 | Uncommon | |
| 33 | Metang | Pokémon - Stage 1 | 80 | Uncommon | |
| 34 | Minun | Pokémon - Basic | 60 | Uncommon | |
| 35 | Numel | Pokémon - Basic | 60 | Uncommon | |
| 36 | Plusle | Pokémon - Basic | 60 | Uncommon | |
| 37 | Poliwhirl | Pokémon - Stage 1 | 80 | Uncommon | |
| 38 | Pupitar | Pokémon - Stage 1 | 70 | Uncommon | |
| 39 | Pupitar | Pokémon - Stage 1 | 80 | Uncommon | |
| 40 | Seadra | Pokémon - Stage 1 | 80 | Uncommon | |
| 41 | Tauros | Pokémon - Basic | 90 | Uncommon | |
| 42 | Wartortle | Pokémon - Stage 1 | 80 | Uncommon | |
| 43 | Aipom | Pokémon - Basic | 50 | Common | |
| 44 | Beldum | Pokémon - Basic | 60 | Common | |
| 45 | Buizel | Pokémon - Basic | 60 | Common | |
| 46 | Carnivine | Pokémon - Basic | 80 | Common | |
| 47 | Cherubi | Pokémon - Basic | 50 | Common | |
| 48 | Chinchou | Pokémon - Basic | 60 | Common | |
| 49 | Horsea | Pokémon - Basic | 50 | Common | |
| 50 | Larvitar | Pokémon - Basic | 50 | Common | |
| 51 | Larvitar | Pokémon - Basic | 60 | Common | |
| 52 | Magmar | Pokémon - Basic | 70 | Common | |
| 53 | Mankey | Pokémon - Basic | 50 | Common | |
| 54 | Misdreavus | Pokémon - Basic | 50 | Common | |
| 55 | Natu | Pokémon - Basic | 50 | Common | |
| 56 | Onix | Pokémon - Basic | 90 | Common | |
| 57 | Onix | Pokémon - Basic | 90 | Common | |
| 58 | Poliwag | Pokémon - Basic | 50 | Common | |
| 59 | Remoraid | Pokémon - Basic | 50 | Common | |
| 60 | Riolu | Pokémon - Basic | 60 | Common | |
| 61 | Roselia | Pokémon - Basic | 60 | Common | |
| 62 | Spearow | Pokémon - Basic | 50 | Common | |
| 63 | Squirtle | Pokémon - Basic | 60 | Common | |
| 64 | Stantler | Pokémon - Basic | 70 | Common | |
| 65 | Teddiursa | Pokémon - Basic | 60 | Common | |
| 66 | Tropius | Pokémon - Basic | 80 | Common | |
| 67 | Turtwig | Pokémon - Basic | 50 | Common | |
| 68 | Vulpix | Pokémon - Basic | 60 | Common | |
| 69 | Weedle | Pokémon - Basic | 40 | Common | |
| 70 | Zubat | Pokémon - Basic | 50 | Common | |
| 71 | Cheerleader's Cheer | Trainer - Supporter | Uncommon | ||
| 72 | Dual Ball | Trainer - Item | Uncommon | ||
| 73 | Emcee's Chatter | Trainer - Supporter | Uncommon | ||
| 74 | Energy Returner | Trainer - Item | Uncommon | ||
| 75 | Engineer's Adjustments | Trainer - Supporter | Uncommon | ||
| 76 | Good Rod | Trainer - Item | Uncommon | ||
| 77 | Interviewer's Questions | Trainer - Supporter | Uncommon | ||
| 78 | Judge | Trainer - Supporter | Uncommon | ||
| 79 | Life Herb | Trainer - Item | Uncommon | ||
| 80 | PlusPower | Trainer - Item | Uncommon | ||
| 81 | Pokémon Circulator | Trainer - Item | Uncommon | ||
| 82 | Rare Candy | Trainer - Item | Uncommon | ||
| 83 | Super Scoop Up | Trainer - Item | Uncommon | ||
| 84 | Crobat | Pokémon - Stage 2 | 130 | SuperRare Holo | |
| 85 | Kingdra | Pokémon - Stage 2 | 130 | SuperRare Holo | |
| 86 | Lanturn | Pokémon - Stage 1 | 110 | SuperRare Holo | |
| 87 | Steelix | Pokémon - Stage 1 | 140 | SuperRare Holo | |
| 88 | Tyranitar | Pokémon - Stage 2 | 160 | SuperRare Holo | |
| 89 | Ursaring | Pokémon - Stage 1 | 110 | SuperRare Holo | |
| 90 | Entei & Raikou LEGEND | Pokémon - LEGEND | 140 | Rare Holo LEGEND | |
| 91 | Entei & Raikou LEGEND | Pokémon - LEGEND | 140 | Rare Holo LEGEND | |
| 92 | Raikou & Suicune LEGEND | Pokémon - LEGEND | 160 | Rare Holo LEGEND | |
| 93 | Raikou & Suicune LEGEND | Pokémon - LEGEND | 160 | Rare Holo LEGEND | |
| 94 | Suicune & Entei LEGEND | Pokémon - LEGEND | 160 | Rare Holo LEGEND | |
| 95 | Suicune & Entei LEGEND | Pokémon - LEGEND | 160 | Rare Holo LEGEND |